The primary goal of CLOUD is to understand the influence of galactic cosmic rays (GCRs) on aerosols and clouds, and their implications for climate.
- Measurement–model comparison of stabilized Criegee intermediate and highly oxygenated molecule production in the CLOUD chamber (Sarnela et al., 2018)
- "Global atmospheric particle formation from CERN CLOUD measurements", http://science.sciencemag.org/content/early/2016/10/26/science.aaf2649"
- "Reduced anthropogenic aerosol radiative forcing caused by biogenic new particle formation" http://www.pnas.org/content/early/2016/10/05/1602360113?trendmd-shared=0
- "Ion-induced nucleation of pure biogenic particles" http://www.nature.com/nature/journal/v533/n7604/full/nature17953.html
- "The role of low-volatility organic compounds in initial particle growth in the atmosphere", http://www.nature.com/nature/journal/v533/n7604/full/nature18271.html
- "The effect of acid–base clustering and ions on the growth of atmospheric nano-particles", http://www.nature.com/ncomms/2016/160520/ncomms11594/full/ncomms11594.html
Atmospheric aerosols and their effect on clouds are poorly understood and yet important for climate. Indeed, they are recognised by the Intergovernmental Panel on Climate Change (IPCC 2013) as the largest source of uncertainty in present radiative forcing and in climate projections over the 21st century. Although its design is optimised to address the cosmic ray question, CLOUD is the first experiment to reach the demanding technological performance and ultralow contaminant levels necessary to be able to measure aerosol nucleation and growth under controlled conditions in the laboratory. Consequently CLOUD has become the world’s leading laboratory experiment to address not only the influence of cosmic rays on aerosol-cloud processes but also more general and equally poorly understood aspects.
At the heart of the experiment is a stainless steel chamber of volume 26m3. This is surrounded by state of the art instrumentation measuring the gases and particles inside. The chamber is filled with synthetic air made from liquid nitrogen and liquid oxygen. Small quantities of other gases such as sulphur dioxide or organic compounds are added, and aerosol particles are formed and characterised.
Experiments often focus on measuring the rate of formation of aerosol particles with different mixtures of gases in the chamber, and investigating the effect of ionisation on this formation rate. The ionisation produced by cosmic rays can be enhanced with a high energy particle beam from the CERN Proton Synchrotron, or removed with a strong electric field. In addition, if the humidity inside the chamber is close to 100%, cooling achieved by fast adiabatic expansion can be used to make clouds in the chamber. At warm temperatures, this allows chemical processes inside cloud droplets to be studied and, at lower temperatures, experiments on ice microphysics are carried out.